Geological and geochemical features of the Dadengge gold polymetallic deposit in Jiaodong Peninsula
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摘要: 本文介绍了大邓格金多金属矿床地质特征,对矿床主量元素、硫同位素、氢-氧同位素及流体包裹体作了测试分析,总结了矿床地球化学特征,讨论了成矿物质来源及成矿物理化学条件。主量元素分析表明蚀变过程中SiO2、K2O含量增高,Na2O、Al2O3、CaO等含量降低;硫同位素组成δ34SCDT值为7.0‰~7.1‰,指示硫可能来自于均一化程度较高的统一流体库;氢同位素组成δ DV-SMOW变化范围较大,为-83.68‰~-116.95‰,氧同位素组成δ18O水值为-2.57‰~8.35‰,显示了成矿流体以岩浆水与大气降水组成的混合水为主;成矿流体主要为中温(86~429℃)、低盐度(1.74%~22.38%NaCleq),属CO2-H2O-N2-NaCl体系。成矿期流体表现出多期、多来源特征,体系物理化学条件的改变和流体的不混溶是导致金等成矿元素沉淀和富集的重要机制。Abstract: In this paper, the authors described the geological features of the the Dadengge gold polymetallic deposit, analyzed major elements, REE, sulfur isotope, δDV-SMOW-δ18OH2O, and fluid inclusions, and then summarized the geochemical features so as to find the ore-forming genesis and physicochemical conditions. Major element analyses show that the alteration zone gained SiO2, K2O but lost Na2O, Al2O3, CaO during alteration. The sulfur isotope composition ranges between 7.0‰ and 7.1‰ δ34SCDT, suggesting that the sulfurs were of the same origin, being a unified source. The δDV-SMOW values range from -83.68‰ to -116.95‰, and theδ18OH2O values range from -2.57‰ to 8.35‰, suggesting that the mineralizing fluids were derived from the mixed magmatic and meteoric water. The mineralizing process took place under the condition of medium temperature (86-429℃) and low salinity (1.74%-22.38% NaCleq), and the mineralizing fluid might have been a CO2-H2O-N2-NaCl system. The mineralizing fluids of the main mineralization stage exhibited feature of multiple sources, and the change of physicochemical conditions and fluid immiscibility were the important mechanisms for deposition and enrichment of gold and other mineralizing elements.
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图 1 胶东东部伟德山地区区域地质矿产简图（据文献[4]修改）
1—中生代白垩纪青山群（以安山岩为主）；2—古元古代荆山群；3—新元古代晋宁期花岗岩；4—新元古代晋宁期花岗闪长岩；5—中生代燕山期伟德山序列崮庄单元细粒辉石角闪石英二长闪长岩；6—中生代燕山期伟德山序列洛西头单元含粗斑中粒角闪黑云石英二长岩；7—中生代燕山期伟德山序列大水泊单元疏粗斑中粒含黑云角闪石英二长岩；8—中生代燕山期伟德山序列不落耩单元疏巨斑中粗粒含角闪石英二长岩；9—中生代燕山期伟德山序列崖西单元疏粗斑中粒含角闪二长花岗岩；10—中生代燕山期伟德山序列虎头石单元细粒二长花岗岩；11—石英闪长玢岩；12—闪长玢岩；13—花岗斑岩；14—二长斑岩；15—岩性/地层界线；16—断层及产状；17—伟德山岩体出露外界线；18—铜/钼/铅/锌/银/金矿床(点)
Figure 1. Simplified geological map and distribution of main nonferrous metal deposit in the eastern area of Jiaodong Peninsula (modified after reference [4])
1-Mesozoic Cretaceous Qingshan Group (andesite);2-Paleoproterozoic Jingshan Group;3-Neoproterozoic Jinning period granite; 4-Neoproterozoic Jinning period granodiorite;5-Mesozoic YanshanianWeideshan granite series:Guzhuang unit,monzonitic diorite; 6-Luoxotou unit,adamellite;7-Dashuipo unit,adamellite;8-Buluojiang unit,adamellite;9-Yaxi unit;10-Hutoushi unit,monzonitic granite; 11-Porphyritic quaitzdiorite;12-Porphyritic diorite;13-Granophyre;14-Porphyritic monzonite;15-Geological boundary; 16-Fault and its attitude;17-Boundary ofWeideshan granite;18-Copper/molybdenum/lead/zinc/silver/gold deposits (ore spots)
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图 2 大邓格金多金属矿区域地质图（据文献[1]修改）
1—新生代第四系；2—古元古代荆山群定国寺段透辉石大理岩；3—古元古代荆山群安吉村段二云石英片岩；4—古元古代荆山群安吉村段黑云片岩；5—中生代白垩纪伟德山序列崮庄单元片麻状细粒辉石石英闪长岩；6—新元古代荣成片麻岩套威海单元条带状细粒含黑云二长花岗质片麻岩；7—新元古代荣成片麻岩套泊于单元条纹状中细粒含角闪黑云花岗闪长岩质片麻岩；8—中元古代长城纪海阳所组合老黄山单元变辉长辉绿岩、斜长角闪岩；9—中元古代长城纪海阳所组合通海单元蛇纹岩、含橄榄透闪石岩；10—石英脉；11—石英闪长玢岩；12—煌斑岩；13—黄铁绢英岩化碎裂岩；14—勘查区范围
Figure 2. Regional geological map of the Dadengge gold polymetallic deposit (modified after reference [1])
1-Cenozoic Quaternary;2-Proterozoic Jingshan Group Dingguosi Member:diopside marble;3-Proterozoic Jingshan Group Anjicun Member: two-mica quartz schist;4-Proterozoic Jingshan Group Anjicun Member:biotite schist;5-Mesozoic CretaceousWeideshan granite series Guzhuang unit:gneissic granule pyroxene quartz diorite;6-Proterozoic Rongcheng bandedWeihai Unit:stripped granule monzonitic granitic gneiss including biotite;7-Proterozoic Rongcheng banded Poyu Unit:striated medium-granule biotite granodioritic gneiss including amphibole; 8-Proterozoic Changcheng period Haiyangsuo Combination Laohuangshan Unit:meta-gabbro,diabase,plagioclase amphibolite;9-Proterozoic Changcheng period Haiyangsuo Combination Tonghai Unit:serpentinite,tremolite rock including olivine;10-quartz;11-Quartz dioriteporphyrite; 12-Lamprophyre;13-Cataclasite with pyritization,sericitization and greisenization;14-Faults;15-Range of exploratory area
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图 3 大邓格金多金属矿区地质图（据文献[1]修改）
1—第四系；2—大理岩；3—黑云片岩；4—花岗闪长质片麻岩；5—斜长角闪岩；6—石英闪长玢岩；7—闪长玢岩；8—煌斑岩；9—黄铁绢英岩化碎裂岩；10—矿脉编号；11—钻孔；12—勘探线及编号
Figure 3. Simplified geological map of the Dadengge gold polymetallic deposit (modified after reference [1])
1- Quaternary;2-Marble;3-Biotite schist;4-Granodioritic gneiss;5-Plagioclase amphibolite;6-Quartz diorite-porphyrite;7-Diorite-porphyrite;8-Lamprophyre;9-Cataclasite with pyritization,sericitization and greisenization;10-Serial number of the mineral vein;11-Drill hole;12-Exploration line and its serial number
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图 4 大邓格金多金属矿床8号勘探线地质剖面图（据文献[1]修改）
1—第四系；2—大理岩；3—斜长角闪岩；4—花岗闪长质片麻岩；5—煌斑岩；6—黄铁绢英岩化碎裂岩；7—金矿体；8—银矿体；9—铅矿体；10—锌矿体；11—铜矿体；12—地质界线；13—钻孔
Figure 4. Geological section along No. 8 exploration line in the Dadengge gold polymetallic deposit (modified after reference [1])
1-Quaternary; 2-Marble; 3-Plagioclasic amphibolite; 4-Granodioritic gneiss; 5-Lamprophyre; 6-Cataclasite with pyritization, sericitization and silicification; 7-Gold orebody; 8-Silver orebody; 9-Lead orebody; 10-Zinc orebody; 11-Copper orebody; 12-Geological boundary; 13-Drill hole
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图 5 大邓格金多金属矿床矿石及显微照片
Py—黄铁矿；Ccp—黄铜矿；Pyr—磁黄铁矿；Qz—石英；Ser—绢云母；Gn—方铅矿；Sp—闪锌矿；Ele—银金矿；a—黄铁绢英岩化碎裂岩型矿石（内有石英脉）（金-银-铜-铅-锌共生），ZK802，221 m；b—黄铁矿石英脉型矿石（铅-铜-金-银共生），ZK604，140 m；c—方铅矿（他形）沿黄铁矿、磁黄铁矿、石英晶隙嵌布；d—黄铜矿微粒以不混溶体被包于闪锌矿之中（乳浊状），或呈他形粒状集合体产出；e—银金矿沿磁黄铁矿与石英和绢云母边缘嵌布；f—闪锌矿、方铅矿（他形）与黄铁矿、磁黄铁矿（半自形）共生
Figure 5. Micrograph of ores in the Dadengge gold polymetallic deposit
Py-Pyrite;Ccp-Chalcopyrite;Pyr-Pyrrhotite;Qz-Quartz;Ser-Sericite;Gn-Galena;Sp-Sphalerite;Ele-Electrum;a-Cataclasite type ore with pyritization,sericitization and silicification (quartz included)(composite orebody of Au-Ag-Cu-Pb-Zn),ZK802,221 m;b-Pyrite and quartz vein type ore (composite orebody of Pb-Cu-Au-Ag),ZK604,140 m;c-Galena (allotriomorphic) distributed along crystals'slits of pyrite,pyrrhotite, quartz;d-Chalcopyrite inlaid in sphalerite (opacification),or exhibiting allotriomorphic granular aggregation;e-Electrum inlaid along edge of quartz and sericite;f-Sphalerite and galena (allotriomorphic) associated with pyrite and pyrrhotite (subhedron)
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图 9 大邓格金多金属矿床流体包裹体特征
a—石英中成群分布的包裹体；b—方解石中成群分布的包裹体；c—石英中无色-灰色Ⅰ型富液相包裹体；d—石英中深灰色Ⅱ型CO2两相包裹体；e—石英中Ⅲ型H2O-CO2三相包裹体；f—方解石中无色-灰色Ⅰ型富液相包裹体
Figure 9. Characteristics of fluid inclusions in the Dadengge gold polymetallic deposit
a-Inclusion group in quartz;b-Inclusion group in calcite; c-Ⅰ type rich liquid inclusions in quartz; d-Ⅱtype V CO2-L CO2 inclusions in quartz;e-Ⅲ type rich H2O-CO2 three-phase inclusions in quartz; f-Ⅰ type rich liquid inclusions in calcite
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图 10 大邓格矿石英及方解石中流体包裹体样品均一温度（a）和盐度（b）分布直方图
Figure 10. Histograms of homogenization temperature (a) and salinity (b) for quartz and calcite fluid inclusions in the Dadengge gold polymetallic deposit
表 1 大邓格金多金属矿床矿石及围岩主量元素分析结果（%）
Table 1 Major element content of orebodies and country rocks in the Dagengge gold polymetallic deposit
序号 样品编号 取样位置/m 岩性 Si02 ai2o3 Fe203 FeO MgO CaO Na20 K20 MnO Ti02 P2O5 烧失量 总和 1 ZK805-1 414.30 矿石 SJH 61.15 0.81 12.25 9.72 2.94 15.51 0.13 0.02 1.57 0.04 0.14 5.33 109.61 2 ZK808-1 262.60 SJH 74.95 12.93 1.84 1.34 0.64 1.75 0.48 5.42 0.09 0.34 0.08 1.43 101.29 3 ZK1002-1 266.50 SJH 79.06 4.82 4.16 0.72 0.66 4.42 0.08 1.55 0.05 0.32 0.30 4.51 100.65 4 ZK805-2 481.20 围岩 πγ 71.71 14.24 1.42 0.57 0.31 0.67 4.12 5.88 0.08 0.21 0.07 1.27 100.55 5 DDG-17 地表 νηδ 56.98 16.72 6.60 3.81 4.67 6.77 4.04 2.29 0.10 0.65 0.38 0.79 103.80 6 WH-1 外围 ηγ 71.90 13.65 1.01 1.87 0.60 1.54 4.01 3.83 0.06 0.27 0.09 0.36 99.19 7 PYJ-1 外围 γδ 64.30 15.46 2.75 3.52 1.85 4.43 3.85 2.09 0.15 0.46 0.10 - 98.96 注：SJH—黄铁绢英岩化碎裂岩；πγ—斑状花岗岩；νηδ—辉石二长闪长岩；ηγ—条带状片麻状细粒黑云二长花岗岩；γδ—条纹片麻状中细粒含角闪黑云花岗闪长岩；6号样引自文献[5]；7号样引自文献[6]。 
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表 2 大邓格金多金属矿床硫同位素组成
Table 2 Sulfur isotope composition of the Dadengge gold polymetallic deposit
序号 样品编号 取样位置/m 矿体编号 岩性 测试对象 δ34Sv.cdt‰ 1 ZK604-1 134.00 锌矿体 绢英岩化碎裂岩 闪锌矿 7.0 2 ZK803 85.00 铅锌矿体 花岗质碎裂岩 闪锌矿 7.1
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表 3 大邓格金多金属矿床及胶东典型金矿床氢-氧同位素组成表
Table 3 Hydrogen and oxygen isotope composition of the Dadengge deposit and the typical gold deposits in Jiaodong
矿床 样品编号 取样位置/m 测试矿物 岩性 δDv_smow‰ δ18Ov.smow‰ δ180水‰ 数据来源 大邓格金多金属矿床 ZK804-l-a 328.70 石英 SJH -92.50 16.00 8.35 本文 ZK804-2-a 342.50 石英 SJH -91.30 13.20 5.57 ZK805-l-a 414.30 石英 SJH -101.80 5.00 -2.57 ZK1002-l-a 266.50 石英 SJH -92.10 8.60 1.01 焦家深部金矿床 ZK634 石英 SγJH -90.16 12.88 4.95 文献[19] ZK615-6 石英 SJH -92.76 13.24 5.31 ZK634-9 石英 SγJH -83.68 12.04 4.11 ZK622-3 石英 SJH -116.96 16.28 8.35 ZK667-11 石英 SγJH -91.38 13.04 5.11 ZK622-5 石英 SγJH -87.15 12.45 4.52 玲珑金矿床 石英 -85.00 13.60 4.20 文献[20] 石英 -76.00 14.10 4.00 石英 -93.00 12.60 3.20 石英 -76.00 13.70 4.30 石英 -62.00 13.20 3.80 文献[21] 石英 -64.00 12.20 6.10 石英 -54.00 16.60 7.20 石英 -58.00 15.00 7.20 玲珑花岗岩 花岗岩全岩 γ -68.40 8.30 4.70-7.60 文献[22 郭家岭花岗岩 花冈石全石 γ -62.40 10.10 7.10 9.10
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表 4 大邓格金多金属矿床流体包裹体显微测温结果
Table 4 Microthermometric data of fluid inclusions in the Dadengge gold polymetallic deposit
样号 岩石类型 取样位置 测试矿物 包裹休类型 气液比/% ThCO2/°C Th/°C 盐度/(%NaCl) 密度/(g/cm3) 富液相包裹体 10~30 283~321 4.8~12.42 0.74~0.87 ZK804-1 SJH 342.50 m Ⅰ-6号矿体 石英 CO2两相包裹体 30 31.60 H2O-CO2三相包裹体 30~80 28.20~31.00 282~360 4.87~12.45 0.65~0.89 富液相包裹体 20~40 212~412 4.26~11.75 0.66—0.94 ZK808-2 SJH 269.60m I-6号矿体 石英 CO2两相包裹体 40~60 26.00~29.20 H2O-CO2三相包裹体 20~60 23.60~28.60 280~429 4.14~11.65 0.68~0.77 ZK808-4 SJH 273.60 m Ⅰ-2号矿体 方解石 富液相包裹体 5~10 86~126 9.08~14.97 1.00—1.07 石英 富液相包裹体 10 255 22.38 1.00 ZK1005-1 SJH 226.80 m Ⅰ-2号矿体 石英 富液相包裹体 8~20 96~129 1.74~4.96 0.97—0.98 ZK1002-1 SJH 266.50 m Ⅰ-2号矿体 石英 富液相包裹体 5~20 142~317 2.07~20.45 0.76~1.08
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表 5 大邓格金及多金属矿床流体包裹体气相成分表
Table 5 Gas phase composition of inclusions in the Dadengge gold polymetallic deposit
样品编号 测试矿物 源石 含量/10-6 h2 n2 CO ch4 CO2 H2O(气相） ZK804-1 石英 黄铁绢英岩化碎裂岩 0.81 1.12 0.25 0.24 17.56 1.76×105 ZK1002-1 石英 黄铁绢英岩化碎裂岩 0.17 3.01 0.21 0.29 3.37 3.93×104
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